A new method to make an all-fiber nonlinear optic device for laser pulse generation is developed by depositing multi-layer graphene oxide (GO) selectively onto the core of the cleaved fiber facet by combining the electrical arc discharge and the laser-driven self-exfoliation. Using the GO colloid droplet with sub-nanoliter volume, we obtained a GO bulk layer deposited on a fiber facet of the order of milliseconds by using an electric arc. The prepared fiber facet was then included in an Er-doped fiber laser (EDFL) cavity and we obtained a few layers of GO having nonlinear optic two-dimensional (2D) characteristics selectively on the fiber core by the laser-driven self-exfoliation. The 2D GO layers on the fiber core served as a stable and efficient saturable absorber enabling robust pulse train generation at λ=1600.5nm, the longest Q-switched laser wavelength in EDFLs. Pulse characteristics were analyzed as we varied the pump power at λ=980nm from 105.2 mW to 193.6 mW, to obtain the maximum repetition rate of 17.8 kHz and the maximum output power of 2.3 mW with the minimum pulse duration of 7.8 μs. The proposed method could be further applied to other novel inorganic 2D materials opening a window to explore their novel nonlinear optic laser applications.

A unique all-fiber interferometric sensor was proposed and successfully demonstrated efficient low-refractive-index liquid sensing in the range from 1.33 to 1.37, which is compatible with those of bio-liquids. A special silica coreless optical fiber with an open V-groove was used as an optical sensing medium, which provided a high sensitivity for a minute liquid volume in the nanoliter scale. The V-groove fiber (VGF) was serially concatenated between two single-mode fibers (SMFs). The LP₀₁ mode guided along the input SMF excited the higher-order modes in the VGF to generate multimode interference, whose spectrum was transmitted through the output SMF. A single liquid droplet with volume of ～80 nanoliters wet the entire hydrophilic surface of the VGF, and the transmission spectra shifted corresponding to its refractive index in a very linear manner. The sensor also showed a negligible temperature cross-sensitivity in the range 25°C–75°C, which overlaps with the biological temperature window such that the sensitivity of 159.696 nm per refractive index unit (nm/RIU) remained independent of the temperature variation. Modal properties of VGF were thoroughly analyzed numerically, and detailed processes for the sensor fabrication and sensing experiments were reported.

The denaturation of double-stranded deoxyribonucleic acid (ds-DNA) has been well known to break nucleobase bonds, resulting in single-stranded deoxyribonucleic acid (ss-DNA) in solutions, which can recombine to form ds-DNA in a reversible manner. We developed an efficient process to irreversibly maintain various DNA denaturation levels in thin solid films in order to investigate the impacts of the denaturation on the optical properties of DNA films. By adding NaOH in an aqueous solution of salmon testis DNA, we flexibly controlled the level of denaturation in the solution, which was then spin-coated on Si and silica substrates to irreversibly bind ss-DNAs in a thin solid film. The denaturation of DNA in thin solid films was experimentally confirmed by ultraviolet-visible and Fourier transform infrared spectroscopic investigations, whose level could be controlled by the NaOH content in the aqueous solution precursor. By this irreversible denaturation process, we developed a new method to flexibly vary the refractive index of DNA thin solid films in a wide range of Δn>0.02 in the visible to near-infrared range. Thermo-optic coefficients dn/dT of the films were also experimentally measured in the temperature range from 40°C to 90°C to confirm the significant impacts of denaturation. Detailed thin film processes and optical characterizations are discussed.